Citation Link: https://doi.org/10.1088/2053-1583/ad5737
Dislocation-free two-dimensional concentric lateral heterostructures: MoS2–TaS2/Au(111)
Publication Type
Article
Subjects
Heterojunction
Scanning tunneling microscope
Condensed matter physics
Materials science
Molecular beam epitaxy
Monolayer
Atomic units
Dislocation
Concentric
Transition metal
Lattice (music)
Nanotechnology
Epitaxy
Chemistry
Optoelectronics
Physics
Geometry
Date Issued
2024
Abstract
We prepared two-dimensional concentric lateral heterostructures of the monolayer transition metal dichalcogenides MoS 2 and TaS 2 by reactive molecular beam epitaxy on chemically inert and weakly interacting Au(111). The heterostructures are in a size regime where quantum confinement can be expected. Despite large lattice mismatch a seamless interconnection of the two materials has been achieved, confirming that the semiconducting core is fully enclosed by a metallic border around its circumference. The resulting strain is analyzed on the atomic scale using scanning tunneling microscopy, corroborated by calculations based on empirical potentials and compared to results from finite elements simulations.
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